uhm, no.
You are thinking about a GUI on your PC. Anope modules add/del functionality to Services. 2 TOTALLY different things.
UPDATE:
Let me explain a bit further. an IRC server and Services usually run on a different computer than your regular PC. It's not currently possible for Anope to send the proper data to your PC to create/destroy GUI windows.
IRC Admins are expected to already know basic IRC commands before becoming Admins. so they should already be used to how Services works. You can write a cript in your clients langauge, if your client supports scripting, and generate some popups to perform commands over IRC. To date I don't know of any that exist though. Try google if you are looking for pop-ups.
[Edited on 7-10-2007 by katsklaw]